22-30 July 2021
North-West University
Africa/Johannesburg timezone
More Information Coming Soon

Elastic and Magnetic properties of Tb-MnO based Thin Films

26 Jul 2021, 12:00
15m
Potchefstroom Campus (North-West University)

Potchefstroom Campus

North-West University

Oral Presentation Track A - Physics of Condensed Matter and Materials Physics of Condensed Matter and Materials

Speaker

Mr Geoffrey Mwendwa (School of Physics, Material Physics Research Institute, University of the Witwatersrand, Private Bag 3, 2050, South Africa)

Description

Multiferroic rare-earth composites in thin-film format have shown promising results towards the attainment of strong coupling of ferroic orders (ferroelasticity, ferromagnetism, ferroelectricity, and ferrotoroidicity) at room temperature, which is a key parameter to the realization of low-energy dissipating devices such as solid-state refrigerators, spintronic memory storage, etc. In this work, we have synthesized Tb-MnO based thin films on (001) Si at ambient temperature using radio frequency magnetron (RF) sputtering at 50 W and investigated their elastic and magnetic properties. The elastic properties of the films have been measured by surface Brillouin scattering (SBS) at ambient temperature, optimized, and fitted with data simulated using surface Elastodynamic Green’s function for discrete phonon dispersion in the k//d range of 0–5. By least-squares fitting approach, the measurement uncertainties have been obtained from the Taylor series expansion of the phonon phase velocity dependence on the primary elastic constants (C11 and C44), yielding the optimum values as; C11 = 180 +/- 4.90 GPa and C44 = 43 +/- 0.89 GPa. On the other hand, the magnetic properties of the films have been studied by vibrating sample magnetometry (VSM). The films have been noted to attain ferromagnetic ordering at T<150 K. Spin-glass-like behaviour associated with competing ferromagnetic and antiferromagnetic magnetic ordering has also been observed at T~50 K.

Keywords: Multiferroics, thin-film, elastic constants, ferromagnetism, spin-glass

Apply to be considered for a student ; award (Yes / No)?

Yes

Level for award;(Hons, MSc, PhD, N/A)?

PhD

Primary author

Mr Geoffrey Mwendwa (School of Physics, Material Physics Research Institute, University of the Witwatersrand, Private Bag 3, 2050, South Africa)

Co-authors

Dr Mathe Bhekumusa (School of Physics, Material Physics Research Institute, University of the Witwatersrand) Prof. Dave Billing (School of Chemistry, Molecular Sciences Institute, University of the Witwatersrand) Dr Rudolph Erasmus (School of Physics, Material Physics Research Institute, University of the Witwatersrand) Dr Morgan Madhuku (iThemba LABS (Gauteng), Private Bag 11, Johannesburg, WITS 2050, South Africa) Mr Adam Shnier (School of Chemistry, Molecular Sciences Institute, University of the Witwatersrand) Prof. Daniel Wamwangi (School of Physics, Material Physics Research Institute, University of the Witwatersrand)

Presentation Materials